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Various theories and models have been published that guide the design and development of learning technologies. While these approaches can be useful for promoting cognitive or affective learning outcomes, user-centered design methods and processes from the field of human-computer interaction (HCI) can also be of value to those in the learning design and instructional design and technology (LIDT) community. In this chapter, we present user-centered design, development, evaluation methods, and processes derived from HCI that lead to highly usable technologies promoting positive user experiences. We begin by aligning these methods and processes with theories commonly referenced in the field of LIDT. We then outline specific methodologies that can be applied during the design and development of digital learning environments. The detailed descriptions outline the goals of the various methods and the ideal stage in which to apply the methods; theory and practice are also discussed. Multiple case examples illustrating how the methods can be used in practice are provided.